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August 15, 2026Chemical ReviewsOpen Access

Triarylborane-CatalyzedHomogeneous Molecular TransformationsUsing Organic Reductants

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Authors

OAOluwaseyi Aderemi AjalaACAnil Chauhan正谷正和 谷川

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Overview

Review reveals advances in triarylborane catalysts for organic reductions with diverse hydride donors, highlighting sustainable alternatives to precious-metal systems.

Key Points

  • Summarize advances from 2016 to 2025 in triarylborane-catalyzed homogeneous reductions across diverse organic reductants, catalyst designs, and reaction mechanisms.
  • Surveyed progress in triarylborane structural modifications tuning Lewis acidity and steric environment around the boron center.
  • Evaluated catalytic performance, functional-group tolerance, and stereocontrol across reductant classes including H2, hydrosilanes, Hantzsch esters, and ammonia borane.
  • Highlighted triarylborane designs that retain high catalytic activity in the presence of Lewis bases such as H2O, CO2, and CO.
  • Mapped mechanistic frameworks governing reductant activation and stereoselective control with non-metal hydride donors.
  • Established main-group boron catalysts as sustainable, practical replacements for precious-transition-metal reduction systems.

Cite This Study

Ajala et al. (2026) studied this question.

synapsesocial.com/papers/6a801a0e75c2e31742c86777https://doi.org/10.1021/acs.chemrev.6c00439
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