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November 29, 2012Angewandte Chemie

A Visible‐Light‐Harvesting Assembly with a Sulfocalixarene Linker between Dyes and a Pt‐TiO₂ Photocatalyst

Takashi Kamegawa Sachiyo Matsuura Hiroki Seto Hiromi Yamashita

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Abstract

Die Verankerung kationischer Farbstoffmoleküle (Thiazolorange, TO) auf Pt-TiO2 zur Bildung einer Sammeleinheit für sichtbares Licht gelang durch Modifikation der Pt-TiO2-Oberfläche mit 4-Sulfocalix[4]aren als Linker, was Oberflächenkomplexe lieferte (siehe Bild). Dieses heterogene System ist ein effizienter Photokatalysator für die Wasserstofferzeugung in Gegenwart eines Opferreagens (TEOA=Triethanolamin).

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Kamegawa et al. (2012) studied this question.

synapsesocial.com/papers/6a8037b36394d40ba7cabb58 https://doi.org/10.1002/ange.201206839

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