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The first catalytic asymmetric three-component allylation of aldimines has been developed. In the presence of L-ramipril acid-oriented N,N′-dioxide–ScIII complex catalyst, a range of homoallylic amines were formed in excellent enantioselectivities (up to 97 % ee) with good yields from corresponding aldehydes, 2-aminophenol and allyltributyltin (see scheme).
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Li et al. (2008) studied this question.
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