A study of striking structural differences in the magic angle of Py2S and coligand effects has been carried out. [Co(Py2S)2Cl2]n is the first integral two-layer interwoven sheet without any counterion or solvate whereas [Co(Py2S)2(NCS)2]n affords a double-stranded linear infinite structure. Thermal analyses of the complexes over the temperature range 25−430 °C show the significant thermal behaviors associated with the structure.
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Jung et al. (1998) studied this question.
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