Raman spectra of cesium triborate were recorded at room temperature and liquid nitrogen temperature and the infrared reflectance spectra at room temperature. The assignments of characteristic vibrational modes are presented. A comparison of cesium borate and lithium borate was made. A correlation exists between the LO–TO splittings of vibrational modes of borate crystals and their non-linear optical efficiencies.
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Wang et al. (1999) studied this question.
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