Femtosecond time-resolved CARS (coherent anti-Stokes Raman scattering) and DFWM (degenerate four-wave mixing) experiments on gas-phase iodine molecules were analyzed within time dependent wave-packet calculations. The recorded signals were interpreted using the ro-vibrational quantum dynamics in different electronic states of I2. Thereby various contributions to the induced third-order polarization were related to overlap integrals between wave packets created by absorption and emission processes. This allows for an intuitive interpretation of the temporal variations in the signals.
No takes yet. Share an insight, caveat, or question.
Meyer et al. (2000) studied this question.
Synapse has enriched 2 closely related papers on similar clinical questions. Consider them for comparative context: