Answers are grounded in this paper and cite their sources.
The classical limit of the Wigner–Weyl representation is used to approximate products of bound-continuum matrix elements that are fundamental to many coherent control computations. The range of utility of the method is quantified through an examination of model problems, single-channel Na2 dissociation and multiarrangement channel photodissociation of CH2IBr. Very good agreement with the exact quantum results is found for a wide range of system parameters.
No takes yet. Share an insight, caveat, or question.
McQuarrie et al. (2003) studied this question.
Synapse has enriched 10 related papers. Consider them for comparative context: