A simple model, consisting of ‘two-body’ reactant and product trajectories joined by an instantaneous switch, is proposed for the alkali atom-alkyl iodide rebound reactions. The electronic potential surfaces governing these trajectories are justified in terms of the electron jump model. Encouraging overall agreement is found with extensive molecular beam data for the K, Cs + CH3I reactions.
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Grice et al. (1971) studied this question.
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