Matrix isolation spectra of the system NH2NH2:N2 were obtained in the region 4000–270 cm—1 at 4.2°K. Spectra taken in this manner are free of complications due to association, over-all rotation, etc. The unusual features of these spectra are that the bands usually assigned to the bending modes which are present in gas-phase spectra at ∼1500–1600 cm—1 are not found; and, that the torsional mode is apparently split. Anomalous behavior for the 6.3-μ gas-phase band was observed.
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Catalano et al. (1963) studied this question.
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