A preliminary investigation of the molecular-beam electric resonance spectrum of the metastable a 3Π state of 12C16O is reported. The electric dipole moment observed is 1.38±0.02 D. The variation of dipole moment with vibrational state appears to be less than 0.005 D per vibration. Lambda doubling values in the Ω=2 fine structure component are reported for J=2, 3, and 4. The population distribution among vibrational states resulting from excitation by 11-V electrons is in good agreement with calculated Franck—Condon factors.
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Freund et al. (1965) studied this question.
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