We study the ultrafast dynamics of clusters immediately after the photodetachment of by performing molecular dynamics simulations based on a microscopic electronic theory. We determine the time scale for the change from the linear (initial situation) to a triangular structure (potential minimum) of the ground state of . Our results are in good agreement with experiment. We show how the time dependence of the internal degrees of freedom is reflected in the `pump and probe' signal. Furthermore, we discuss the application of our results to magnetic systems and chemical reactions.
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Jeschke et al. (1996) studied this question.
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