Since our observation that the kinetically stable 1-D 1:1 phase of Fe(C5Me5)+ 5(TCNQ)− exhibits metamagnetic behavior (TN = 2.55°K; HC=1.5 Koe) we have pursued the synthesis of compounds with a ferromagnetic ground state. Several new 1-D Fe(C5Me5)+ 5 substances containing radical anions have been prepared. Each compound exhibits different magnetic properties, and some exhibit slow paramagnetic relaxation (in zero field) suggesting spin on the anions.
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Miller et al. (1985) studied this question.
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