Time-resolved coherent x-ray Raman signals of molecules are computed by formulating the nonlinear response in terms of correlation functions of charge and current densities. Simulations performed on one-dimensional molecular chains demonstrate that Raman resonances provide a direct local probe for valence-excitation dynamics with high spatial and temporal resolutions.
No takes yet. Share an insight, caveat, or question.
Tanaka et al. (2003) studied this question.
Synapse has enriched 5 related papers. Consider them for comparative context: