We propose and demonstrate an efficient sum-frequency mixing scheme based on narrowband and chirped broadband pulses. It combines the advantages of wider spectral acceptance bandwidth and of alleviating the temporal walk-off, which are both beneficial to higher conversion efficiency. Chirped sum-frequency pulses at 455 nm with energy up to 360 µJ, corresponding to a conversion efficiency of ~ 40%, are obtained and the pulses can be compressed to ~ 110 fs. The sum-frequency mixing scheme may provide a promising route to the efficient generation of deep-ultraviolet femtosecond pulses.
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Zhao et al. (2010) studied this question.
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