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Degenerate four-wave mixing in sodium vapor is investigated using a flashlamp-pumped dye laser synchronized on a cw dye laser. At low atomic density, the reflectivity versus the pump intensity and the line shapes are in good agreement with theoretical predictions in the case of both plane waves and Gaussian beams. At high atomic density, reflectivities much higher than unity have been observed. The influence of the pump imbalance has been studied as well as the deformation of the wave front of the conjugated beam introduced by the pump beams. In the high-atomic-density case, the theoretical problem is more complex, and our experimental results exhibit only qualitative agreement with theory.
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Kleinmann et al. (1985) studied this question.
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