We report a method that is able to provide refined structural information on molecular packing in biomolecular assemblies using polarization-resolved four-wave mixing and coherent anti-Stokes Raman-scattering microscopy. These third-order nonlinear processes allow quantifying high orders of symmetry which are exploited here to reveal a high level of detail in the angular disorder behavior at the molecular scale in lipid membranes.
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Bioud et al. (2014) studied this question.
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