A theoretical calculation is made to explain the widths of the isotropic parts of polarized Raman lines in liquids. The calculation is based on the model of the intermolecular resonance-type vibrational relaxation through the vibration-dependent term of the Lennard-Jones atom-atom interaction. The result is applied to the Raman lines of liquid nitrogen, oxygen, and carbon disulfide, and compared with the experimental data.
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Kakimoto et al. (1974) studied this question.
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