A method is presented for probing chemical reaction mechanisms experimentally with perturbations and measurements of the response. Time series analysis and the methods of linear control theory are used to determine the Jacobian matrix of a reaction at a stable stationary state subjected to random perturbations. The method is demonstrated with time series of a model system, and its performance in the presence of noise is examined.
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Mihaliuk et al. (1999) studied this question.
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