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Laser multiphoton ionization (MPI) is used to detect nascent photoproducts following the UV photodissociation of UF6. Sensitivity is high, and there is no measurable background due to the MPI of parent UF6. The technique is very well suited for monitoring isotopically selective photodissociation on a ’’single shot’’ basis.
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Stuke et al. (1981) studied this question.
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