An ABA triblock copolymer with a mechanochemically active gem-dichlorocyclopropane rich polyester block is synthesized via chain extension with polymethylacrylate under SET-LRP conditions. The platform allows for the efficient mechanochemical ring opening of the gDCC groups to 2,3-dichloroalkenes, a promising approach to the synthesis of high mechanophore content polymers with enhanced stability.
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Kean et al. (2012) studied this question.
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