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Two of the 3 Raman-active fundamentals of UF6 have been observed at 666.6±0.3 (ν1) and 535±5 cm—1 (ν2) for a gaseous sample. The new value for ν2 is in good agreement with the value 532 cm—1 obtained earlier by Gaunt from infrared combinations. The sample of UF6 was contained in a Pyrex Raman tube and was irradiated for many hours with 4358 A light with no visible deterioration. Gaunt's thermodynamic functions remain valid.
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Claassen et al. (1956) studied this question.
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