The surface tensions of both simple and complex liquid mixtures are considered. It is shown that the surface tensions of mixtures of simple liquids can be predicted well from a model utilizing the concept of a regular surface solution. For complex mixtures, the use of a parameter reflecting the difference in characteristic energy between the bulk liquid and the surface leads to a good fit of the data for a number of systems.
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Sprow et al. (1967) studied this question.
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