Dimers of flat (EDO-TTF)+ molecules separated by bent neutral EDO-TTF (ethylenedioxytetrathiafulvalene) molecules are found in the insulator phase of (EDO-TTF)2PF6, but not in that of the metallic phase. The cooperativity of Peierls distortion, charge ordering, and anion ordering in this metal–insulator transition can be regarded as the result of a molecular displacement.
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Aoyagi et al. (2004) studied this question.
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