We have measured the light scattering profiles of CO2, N2, C2F6, and C2H6 at 29 °C in both kinetic and hydrodynamic regimes. The generalized theory by Weinberg, Kapral, and Desai was applied for the first time, we believe, to analyze the power spectra of C2F6 and C2H6, for which the Mountain theory was inadequate. We have also observed the rotational relaxation times of C2H6 and C2F6 and the vibrational relaxation time of the latter.
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Lao et al. (1976) studied this question.
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