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An electric analog of the metal‐solution interface was assumed and changes were deduced mathematically for application of a square wave voltage. The analysis was verified using actual electric components, and it was demonstrated that the component of capacity could be measured readily. The method was applied with some success to each of the following systems: mercury in , platinum, silver, copper, aluminum, and tantalum in .
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McMullen et al. (1959) studied this question.
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