Here we introduce for the first time a metal-free trianglamine-based supramolecular organic framework, T-SOF-1, with permanent intrinsic porosity and high affinity to CO 2 . The capability of tuning the pore aperture dimensions is also demonstrated by molecular guest encapsulation to afford excellent CO 2 /CH 4 separation for natural gas upgrading.
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Chaix et al. (2018) studied this question.
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