The visible absorption spectra of the ions [Fe(CN)5NO]2—, [Mn(CN)5NO]3—, and [Cr(CN)5NO]3— are interpreted using a crystal field level scheme of C4v symmetry. Assuming a strong axial compression to be present a self-consistent assignment is obtained for both the 3d5 and 3d6 electronic configurations.
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Gray et al. (1962) studied this question.
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