The MgCH3 radical was produced by a laser ablation/photolysis technique in a cold supersonic free-jet expansion and probed by laser induced fluorescence. Rotationally resolved spectra for both spin-orbit components of the à 2E←X̃ 2A1 electronic transition have been recorded. The analysis of these spectra yields the rotational constants of MgCH3 and therefrom a structure for the radical is proposed. A comparison is made among a series of alkyl organometallic radicals.
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Rubino et al. (1995) studied this question.
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