Selective photodissociation of TlCl and TlI using 248 nm radiation from a KrF* excimer laser has been used to create a Tl* (6p²P3/2) metastable state population inversion. Stimulated anti-Stokes Raman emission at 376 nm has been observed using a 532 nm pump laser. Output power at the anti-Stokes wavelength and conversion efficiencies are reported.
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White et al. (1982) studied this question.
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