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The first observation of nonresonant, stimulated anti-Stokes Raman emission is reported. A metastable Tl(6p²P3/2ᵒ) inversion is created by selective photodissociation of TlCl. Raman scattering from the Tl metastable state to ground using 532- and 355-nm pump lasers resulted in stimulated emission at 376 and 278 nm, respectively. Conversion efficiencies up to 10% are reported.
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White et al. (1982) studied this question.
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