Polymerization—a single molecule view: Molecular motion of free and incorporated single perylene diimide derivatives during radical polymerization of styrene and styrene networks, studied by a combination of fluorescence correlation spectroscopy and wide-field microscopy, can be observed over the entire conversion range from free diffusion to immobilization of the dyes. In particular, the presence of evolving heterogeneities could be visualized.
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Wöll et al. (2007) studied this question.
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