Stable free radicals can be trapped inside a three-dimensional (3D) inorganic network. The formation of a new type of mixed-metal oxalate [MnII(H2O)CrIII(ox)3]− is induced by the presence of a cationic nitronyl nitroxide radical (rad+). The figure shows a stylized view of the 3D network ○ = Mn, • = Cr). This hybrid organic–inorganic compound behaves as an antiferromagnet at 6 K.
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Ballester et al. (2001) studied this question.
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