The Brillouin lines in the polarized light scattering spectrum of liquid CCI4, SiCl4 and SnCl4 were analysed and relaxation times and relaxation strengths were calculated in the temperature range between the melting and the boiling points of these liquids. The results were interpreted on the basis of an isolated binary collision model. The connection between experimental relaxation times, theoretical relaxation probabilities and molecular collision numbers as obtained from model considerations are discussed. The relative significance of factors as the anisotropy of intermolecular forces and multiple collision is assessed.
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Samios et al. (1980) studied this question.
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