A multilayer film was simulated by number, volume, and temperature ensembles. Systems of 224 and 672 molecules were scaled to methane and argon-graphite parameters. Studies were done at T=25 K for the coverages of 0.90 to 4.13({}3 ×{} {}3 ) monolayers. The layers within the film are incommensurate in the methane but commensurate for the argon case. For methane, the first two layers are mutually modulated by rotated misfit dislocations.
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Hruska et al. (1988) studied this question.
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