Infrared and Raman spectra of carbon subsulfide (C3S2) in various phases have been obtained in the region 30–4000 cm−1. Mass and ultraviolet spectra are also presented. Analysis of the vibrational spectra indicates a D∞h structure. Of particular interest is the 94-cm−1 band assigned as ν7, the central-carbon bending frequency, which lies at a higher frequency than the analogous band in C3O2. A vibrational analysis has also been performed.
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Smith et al. (1966) studied this question.
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