Polydichlorophosphazene (NPC12)X is unique as a synthetic precursor for poly(organo)phosphazenes [1–6] and presents special problems in polymerization studies because of branching, crosslinking, and cyclization reactions and in characterization due to the polymer's hydrolytic instability. This paper reviews the literature and discusses problem areas and recent advances relating to polydichlorophosphazene polymerization. Melt, solution, and irradiation polymerization reactions and mechanisms are discussed. Previously unpublished results are presented, and current research efforts and areas for future investigation are considered.
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Gary L. Hagnauer (1981) studied this question.
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