The theory of the low-frequency depolarized light-scattering spectra from liquids composed of two components, both of which are symmetric tops, is developed. The rotational motion is assumed to be diffusional, and the expressions for the linewidths are related to the single-particle orientational autocorrelation times. The concentration dependence of these single-particle correlation times is also discussed.
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Kivelson et al. (1975) studied this question.
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