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Single crystals of a new nonlinear optical organic material, 2-cyano-3-(2-methoxyphenyl)-2-propenoic acid methyl ester (CMP-methyl) were grown, and the linear and nonlinear optical properties were investigated in detail. CMP-methyl crystals belong to space group P21, and the lattice parameters are a=4.020 Å, b=9.984 Å, c=13.757 Å, β=92.25° and Z=2. The largest second-order nonlinear optical coefficient was measured to be d 22=29 pm/V. Crystals were of fairly good optical quality.
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Nakatani et al. (1992) studied this question.
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