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Ising-like phenomenological Hamiltonians for coupled lattice processes, such as spin conversion for Fe(II) complexes and concurrent ordering of solvent molecules, are considered. The model is shown to account for experimental data including the temperature dependence of magnetization data, the structural changes associated with spin crossover of magnetically active and silent components of the crystal lattice, and the correlation between the two.
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Chernyshov et al. (2007) studied this question.
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