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We report measurements of the optical properties of deuterated zinc tris thiourea sulfate (d-ZTS). The material is being studied for its potential value in optical frequency conversion and electro-optic applications. The electro-optic and piezoelectric measurements along with those for the dielectric constant indicate that the figure of merit for electro-optic modulation is comparable to that of KDP. However, careful refractive index measurements along with an analysis of the nonlinear coefficient tensor show that d-ZTS will not noncritically phase match for second-harmonic generation despite the promise shown by its undeuterated analog. In addition, the acceptance angle even for critical phase matching is very small.
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Ramabadran et al. (1994) studied this question.
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