We describe an experiment for investigating the 5S1∕2→5D5∕2 two-photon transition in rubidium using a single grating-feedback diode laser operating at 778.1nm (385THz). Continuous tuning of the laser frequency over 4GHz allows for the clear resolution of the Doppler-free spectral features and allows accurate measurement of the hyperfine ground-state splitting. A direct comparison between Doppler-broadened and Doppler-free spectral features is possible because both are distinctly evident in the two-photon spectra. By independently modifying the polarization state of the two laser fields, the impact of electric dipole selection rules on the two-photon transition spectra is investigated. This experiment is a valuable addition to the advanced undergraduate laboratory because it uses much of the same equipment as the single-photon saturated absorption spectroscopy experiment performed on the 5S1∕2→5P3∕2 transition in rubidium (λ=780.24nm) and provides students with an opportunity to investigate characteristics of atomic spectra not evident in the single-photon experiment.
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Olson et al. (2006) studied this question.
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