Triple- and double-photon inelastic and elastic scattering is observed from diamond upon the passage of intense picosecond laser pulses. The spectrum and intensity of the nonlinear scattering is measured. The triple-photon scattering is interpreted in terms of the hyper-Raman and hyper-Rayleigh effects. The value for the three-photon Raman hyperpolarizability is estimated from the experiment.
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Yu et al. (1975) studied this question.
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