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The electron paramagnetic resonance results of three chromium nitrosyl complexes are reported (pentacyano, penta-aquo, and penta-amino). Hyperfine structure with the nucleus of the metal as well as with the nuclei of some of the ligands is observed. We attempt to explain the interaction with the ligand nuclei by mixing the ground state with excited states (charge transfer) by means of the exchange with the unpaired electron. Different possibilities for the configuration of the ground state are discussed.
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Danon et al. (1966) studied this question.
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