An electron dynamics mechanism of charge separation in the initial stage of excited-state reactions of the class of XMnOH2 ⋅⋅⋅A→XMnOH⋅⋅⋅HA (X=OH or OCaH; A=N-methylformamidine, guanidine, imidazole, or ammonia cluster) is reported. The dynamic effect of calcium doping is also revealed. This study provides a novel factor to be considered in designing efficient systems for photoinduced water splitting.
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Yamamoto et al. (2015) studied this question.
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