It is shown that quantum interference with classical beams may be used to suppress or enhance the rate of spontaneous photon-pair production from a nonlinear crystal. Sum-frequency generation of the classical beams is simultaneously enhanced or suppressed via interference with a classical pump. In the extreme case, a crystal which is transparent to individual photons may block all photon pairs, converting them to 2w. This constitutes a coherent nonlinear response at the single-photon level, enhanced by a factor of approximately 10 10 Experimental data and a theoretical description are presented, and an attempt is made to delineate the classical and quantum aspects of these effects.
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Resch et al. (2002) studied this question.
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