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Group theoretical methods are used to construct the [AX]4 nuclear spin hamiltonian for a system with tetrahedral symmetry. This is used to analyse the fluorine and phosphorus spectra of tetrakis (2-fluoro-1,3,2-benzo-dioxaphosphole) nickel(0). Tables are given which will assist the construction of the spin hamiltonian of any tetrahedral spin system.
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R. M. Lynden‐Bell (1968) studied this question.
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