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The probability of preparing multilevel atoms in high-lying levels by multiphoton excitation using one or more laser pulses can be increased by suitably tailoring the pulse amplitudes and frequencies. Few, if any, systematic methods designed specifically for multilevel excitation have been proposed. We present in this paper specific pulses and phase modulations which give specific degrees of inversion of multilevel atoms in analytic form.
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Hioe et al. (1984) studied this question.
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