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A criterion for the choice for the monomer partition model in mathematical modeling of emulsion copolymerization systems is presented. In order to develop this criterion, seeded emulsion copolymerizations of several monomer systems with a wide variety of reactivity ratios and water solubilities were simulated using monomer partition models of different complexity. The simulations included different processes, solids contents and amounts of seed. The criterion for the choice of the monomer partition model was made on the basis of using the simplest but sufficiently accurate model.
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Gugliotta et al. (1995) studied this question.
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