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The population analysis of higher order densities previously described by us and other investigators, has been applied to the description of 1,5—X2B3H3(X=N, CH, P, SiH, BH−) members of the closo-borane family. The calculated results, obtained at the SCF level, suggest the presence of three-center nonclassical bonds in the majority of systems studied. The good agreement between our results and those obtained from more sophisticated methods make this procedure a suitable and simple tool for detecting and localizing three-center bonds.
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Torre et al. (1999) studied this question.
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