Electron–nuclear double resonance (ENDOR) spectra are presented for the odd‐alternate aromatic hydrocarbon neutral radicals phenalenyl, [2H5]phenylphenalenyl and for the benzo[c,d]pyrenyl and benz[d,e]anthracenyl radicals formed by thermal dissociative processes in solution. Proton hyperfine coupling constants were determined from the ENDOR spectra and were shown to give an excellent linear correlation with McLachlan spin densities with Q = −26.5 G.
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Lewis et al. (1985) studied this question.
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